2014: Quantum and semiclassical physics behind ultrafast optical nonlinearity in the midinfrared: The role of ionization dynamics within the field half cycle

Scientists from the Faculty of Physics, Lomonosov Moscow State University, revealed the role of ionization dynamics within the field half cycle in formation of ultrafast optical nonlinearity in the midinfrared.

Ultrafast ionization dynamics within the field half cycle is shown to be the key physical factor that controls the properties of optical nonlinearity as a function of the carrier wavelength and intensity of a driving laser field. The Schrödinger-equation analysis of a generic hydrogen quantum system reveals universal tendencies in the wavelength dependence of optical nonlinearity, shedding light on unusual properties of optical nonlinearities in the midinfrared. For high-intensity low-frequency fields, free-state electrons are shown to dominate over bound electrons in the overall nonlinear response of a quantum system. In this regime, semiclassical models are shown to offer useful insights into the physics behind optical nonlinearity.

The results of this work have been published in the paper: E.E. Serebryannikov and A.M. Zheltikov, “Quantum and semiclassical physics behind ultrafast optical nonlinearity in the midinfrared: The role of ionization dynamics within the field half cycle,” Phys; Rev. Lett. 113, 043901 (2014).